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001-es BibID:	BIBFORM084034
035-os BibID:	(WoS)000392422200021 (Scopus)85007442774
Első szerző:	Csehi András (fizikus)
Cím:	Towards controlling the dissociation probability by light-induced conical intersections / András Csehi, Gábor J. Halász, Lorenz S. Cederbaum, Ágnes Vibók
Dátum:	2016
ISSN:	1359-6640 1364-5498
Megjegyzések:	Light-induced conical intersections (LICIs) can be formed both by standing or by running laser waves. The position of a LICI is determined by the laser frequency while the laser intensity controls the strength of the nonadiabatic coupling. Recently, it was shown within the LICI framework that linearly chirped laser pulses have an impact on the dissociation dynamics of the D+2 molecule (J. Chem. Phys. 143, 014305, (2015); ibid 144, 074309, (2016)). In this work we exploit this finding and perform calculations using chirped laser pulses in which the time dependence of the laser frequency is designed so as to force the LICI to move together with the field-free vibrational wave packet as much as possible. Since nonadiabaticity is strongest in the vicinity of the conical intersection, this is the first step towards controlling the dissociation process via the LICI. Our showcase example is again the D+2 molecular ion. To demonstrate the impact of the LICIs on the dynamical properties of diatomics, the total dissociation probabilities and the population of the different vibrational levels after the dissociation process are studied and discussed.
Tárgyszavak:	Természettudományok Fizikai tudományok idegen nyelvű folyóiratközlemény külföldi lapban folyóiratcikk
Megjelenés:	Faraday Discussions. - 194 (2016), p. 479-493. -
További szerzők:	Halász Gábor J. (1961-) (fizikus) Cederbaum, Lorenz S. Vibók Ágnes (1962-) (fizikus)
Pályázati támogatás:	GOP-1.1.1-12/B-2012-000 Egyéb GINOP-2.3.6-15-2015-00001 GINOP
Internet cím:	Szerző által megadott URL DOI Intézményi repozitóriumban (DEA) tárolt változat
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